Hasil untuk "Plasma physics. Ionized gases"

Roman S. Zemskov, Maxim V. Barkov, Evgeniy S. Blinov et al.

A pioneering detailed comparative study of the dynamics of plasma flows generated by high-power nanosecond and high-intensity femtosecond laser pulses with similar fluences of up to <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mn>3</mn><mo>×</mo><msup><mn>10</mn><mn>4</mn></msup></mrow></semantics></math></inline-formula> J/cm² is presented. The experiments were conducted on the petawatt laser facility PEARL using two types of high-power laser radiation: femtosecond pulses with energy exceeding 10 J and a duration less than 60 fs, and nanosecond pulses with energy exceeding 10 J and a duration on the order of 1 ns. In the experiments, high-velocity (>100 km/s) flows of «femtosecond» (created by femtosecond laser pulses) and «nanosecond» plasmas propagated in a vacuum across a uniform magnetic field with a strength over 14 T. A significant difference in the dynamics of «femtosecond» and «nanosecond» plasma flows was observed: (i) The «femtosecond» plasma initially propagated in a vacuum (no B-field) as a collimated flow, while the «nanosecond» flow diverged. (ii) The «nanosecond» plasma interacting with external magnetic field formed a quasi-spherical cavity with Rayleigh–Taylor instability flutes. In the case of «femtosecond» plasma, such flutes were not observed, and the flow was immediately redirected into a narrow plasma sheet (or «tongue») propagating across the magnetic field at an approximately constant velocity. (iii) Elongated «nanosecond» and «femtosecond» plasma slabs interacting with a transverse magnetic field broke up into Rayleigh–Taylor «tongues». (iv) The ends of these «tongues» in the femtosecond case twisted into vortex structures aligned with the ion motion in the external magnetic field, whereas the «tongues» in the nanosecond case were randomly oriented. It was suggested that the twisting of femtosecond «tongues» is related to Hall effects. The experimental results are complemented by and consistent with numerical 3D magnetohydrodynamic simulations. The potential applications of these findings for astrophysical objects, such as short bursts in active galactic nuclei, are discussed.

Khadija Shabbir, Brian Leard, Zibo Wang et al.

The Multi-Mode Model (MMM) is a physics-based anomalous transport model integrated into TRANSP for predicting electron and ion thermal transport, electron and impurity particle transport, and toroidal and poloidal momentum transport. While MMM provides valuable predictive capabilities, its computational cost, although manageable for standard simulations, is too high for real-time control applications. MMMnet, a neural network-based surrogate model, is developed to address this challenge by significantly reducing computation time while maintaining high accuracy. Trained on TRANSP simulations of DIII-D discharges, MMMnet incorporates an updated version of MMM (9.0.10) with enhanced physics, including isotopic effects, plasma shaping via effective magnetic shear, unified correlation lengths for ion-scale modes, and a new physics-based model for the electromagnetic electron temperature gradient mode. A key advancement is MMMnet’s ability to predict all six transport coefficients, providing a comprehensive representation of plasma transport dynamics. MMMnet achieves a two-order-of-magnitude speed improvement while maintaining strong correlation with MMM diffusivities, making it well-suited for real-time tokamak control and scenario optimization.

Shigeyuki Takagi, Shih-Nan Hsiao, Yusuke Imai et al.

The fabrication of semiconductor devices with three-dimensional architectures imposes unprecedented demands on advanced plasma dry etching processes. These include the simultaneous requirements of high throughput, high material selectivity, and precise profile control. In conventional reactive ion etching (RIE), fluorocarbon plasma provides both accelerated ion species and reactive neutrals that etch the feature front, while the CF<i>_x</i> radicals promote polymerization that protects sidewalls and enhance selectivity to the amorphous carbon layer (ACL) mask. In this work, we present computational results on the role of CF₄ addition to hydrogen fluoride (HF) plasma for next-generation RIE, specifically cryogenic etching. Simulations were performed by varying the CF₄ concentration in the HF plasma to evaluate its influence on ion densities, neutral species concentration, and electron density. The results show that the densities of CF<i>_x</i> (<i>x</i> = 1–3) ions and radicals increase significantly with CF₄ addition (up to 20%), while the overall plasma density and the excited HF species remain nearly unchanged. The results of plasma density and atomic fluorine density are consistent with the experimental observations of the HF/CF₄ plasma using an absorption probe and the actimetry method. It was verified that the gas-phase reaction model proposed in this study can accurately reproduce the plasma characteristics of the HF/CF₄ system. The coupling of HF-based etchants with CF<i>_x</i> radicals enables polymerization that preserves SiO₂ etching throughput while significantly enhancing etch selectivity against the ACL mask from 1.86 to 5.07, with only a small fraction (~10%) of fluorocarbon gas added. The plasma simulation provides new insights into enhancing the etching performance of HF-based cryogenic plasma etching by controlling the CF₂ radicals and HF reactants through the addition of fluorocarbon gases.

Enrico Zio, Enrico Zio, Koroush Shirvan et al.

“We have opinions, we make observations, we change our opinions.” Stephen Senn, Dicing with Death, 2003. The purpose of this review paper is to inform debate and provide snapshot opinions about challenges and solutions for the development of nuclear fission technology. We review the socio-political and techno-economic status of nuclear power technology, which, as almost always during its history, is on an edge from which it may jump to success or fall into the abyss of oblivion. Recent nuclear projects and claims are reviewed in light of lessons learned from the international aircraft and minerals processing industries on manufacturing, construction, and technology maturity. For new nuclear reactor projects and designs, these experiences assist in systematically and objectively quantifying investor risk. We strongly recommend the deployment of nuclear fission for energy production everywhere in the world, depending on the scale and dominant economic factors.

Bianca Schacherl, Kiara Maurer, Martin Schäfer et al.

Targeted alpha therapy (TαT) represents an emerging and cutting-edge treatment option for patients dealing with highly challenging metastatic cancer diseases. Critically, the limited supply of alpha-particle-emitting radionuclides, so-called alpha in vivo nanogenerators, hampers wider utilization of TαT in clinical settings. This could effectively be circumvented by alternative production routes, including straightforward purification and reformulation strategies. Radionuclide generators offering great potential in simple and robust elution strategies can be provided that still adhere to high radioisotopic, radionuclidic, and radiochemical purity criteria. This study takes a first step towards novel separation strategies by providing additional sources of alpha in vivo nanogenerators for TαT through experiments with various metal surrogates. With different systems, 232Th/natBa was used as a radionuclide generator analogue to 227Th/223Ra, and 232Th/natBa/natLa was used as a triplet analogue to 229Th/225Ra/225Ac. Three selective resins (UTEVA, TEVA, DGA-N) were evaluated for the 232Th/natBa system. Two perturbations of the best-performing resin were further evaluated using a larger diameter column and 1 week of equilibration. For the 232Th/natBa/natLa separation system, a combined column with two selective resins (TK200, TK101) was employed and evaluated. The results thus obtained pave the way for alternative separation strategies in radioactive proof-of-concept validation in the near future.

Sagi Turiel, Alexander Gribov, Daniel Maler et al.

Theta Pinch is one of the promising methods for the generation of hot and dense plasma. In this paper, we describe the results of experimental research on a small-scale Theta Pinch created with Helium or Hydrogen plasmas. Different plasma diagnostics, namely, optical, microwave cut-off, laser interferometry, visible spectroscopy, Thomson scattering, and Laser-Induced Fluorescence were used to characterize the time- and space-resolved evolution of the plasma parameters, and the specific features of these diagnostic results obtained are discussed. The measured plasma density and the electron and ion temperature evolution, obtained by these various diagnostic tools, agree to a satisfactory level. These methods will be applied for studies of the parameters of the plasma in the device that is being developed by the nT-Tao company towards fusion energy.

Petr Hoffer, Václav Prukner, Garima Arora et al.

This study utilizes the Kerr effect in the analysis of a pulsed electric field (intensity ~10⁸ V/m, limited by the liquid dielectric strength) in deionized water at the sub-nanosecond time scale. The results provide information about voltage waveforms at the field-producing anode (160 kV peak, d<i>u</i>/d<i>t</i> > 70 kV/ns). The analysis is based on detecting the phase shifts between measured and reference pulsed laser beams (pulse width, 35 ps; wavelength, 532 nm) using a Mach–Zehnder interferometer. The signal-to-noise ratio of the detected phase shift is maximized by an appropriate geometry of the field-producing anode, which creates a correctly oriented strong electric field along the interaction path and simultaneously does not electrically load the feeding transmission line. The described method has a spatial resolution of ~1 μm, and its time resolution is determined by the laser pulse duration.

Tashiema L. Ulrich, Theodore M. Besmann

The phases in uranium-silicide binary system were evaluated in regards to their stabilities, phase boundaries, crystal structures, and phase transitions. The results from this study were used in combination with a well assessed literature to optimize the U-Si phase diagram using the CALPHAD method. A thermodynamic database was developed, which could be used to guide nuclear fuel fabrication, could be incorporated into other nuclear fuel thermodynamic databases, or could be used to generate data required by fuel performance codes to model fuel behavior in normal or off-normal reactor operations. The U3Si2 and U3Si5 phases were modeled using the Compound Energy Formalism model with 3 sublattices to account for the variation in composition. The crystal structure used for the USi phase was the tetragonal with an I4/mmm space. Above 450°C, the U3Si5 phase was modeled. The composition of the USi2 phase was adjusted to USi1.84. The calculated invariant reactions and the enthalpy of formation for the stoichiometric phases were in agreement with experimental data.

Derjew Ayele Ejigu, Yanjie Tuo, Xiaojing Liu

Nuclear power plants produce a massive amount of clean energy and necessitate safe operation through intelligence technologies. Recently, the rapid advancements in communication infrastructures including artificial intelligence, big data computing, and Internet of Things devices moving the nuclear industries towards digitalization and intelligence to improve safety. The integration of these technologies into the nuclear sector offers effective tactics in addressing several challenges in the control and safe operation of nuclear power plants. This can be achieved through the insights generated from massive amounts of data. This paper comprehensively reviews the literature on artificial intelligence technologies and big data, seeking to provide a holistic perspective on their relations and how they can be integrated with nuclear power plants. The utilization of computing platforms boosts the deployment of artificial intelligence and big data analytics effectively in nuclear power plants. Further, this review also points out the future opportunities as well as challenges for applying artificial intelligence and big data computing in the nuclear industry.

Aleksey V. Chaplygin, Elizaveta P. Simonenko, Mikhail A. Kotov et al.

The short-term (5 min) exposure to the supersonic flow of carbon dioxide plasma on ultrahigh-temperature ceramics of HfB₂-30vol.%SiC composition has been studied. It was shown that, when established on the surface at a temperature of 1615–1655 °C, the beginning of the formation of an oxidized layer takes place. Raman spectroscopy and scanning electron microscopy studies showed that the formation of a porous SiC-depleted region is not possible under the HfO₂-SiO₂ surface oxide layer. Numerical modeling based on the Navier–Stokes equations and experimental probe measurements of the test conditions were performed. The desirability of continuing systematic studies on the behavior of ultrahigh-temperature ZrB₂/HfB₂-SiC ceramics, including those doped with various components under the influence of high-enthalpy gas flows, was noted.

Jonathan E. Thomas, Katharina Stapelmann

Cold atmospheric plasmas (CAPs) within recent years have shown great promise in the field of plasma medicine, encompassing a variety of treatments from wound healing to the treatment of cancerous tumors. For each subsequent treatment, a different application of CAPs has been postulated and attempted to best treat the target for the most effective results. These treatments have varied through the implementation of control parameters such as applied settings, electrode geometries, gas flow, and the duration of the treatment. However, with such an extensive number of variables to consider, scientists and engineers have sought a means to accurately control CAPs for the best-desired effects in medical applications. This paper seeks to investigate and characterize the historical precedent for the use of plasma control mechanisms within the field of plasma medicine. Current control strategies, plasma parameters, and control schemes will be extrapolated through recent developments and successes to gain better insight into the future of the field and the challenges that are still present in the overall implementation of such devices. Proposed approaches, such as data-driven machine learning, and the use of closed-loop feedback controls, will be showcased as the next steps toward application.

Jarrod Lewis, Jarrod Lewis, Ross Springell et al.

The different structures and behaviors of UO2+x observed in crystallographic and local structure measurements were examined by extended X-ray absorption fine structure (EXAFS) measurements of pristine UO2.0, p+ and He2+ irradiated UO2.0, and, at multiple temperatures, bulk U4O9 and U3O7 and thin film U4O9-δ on an epitaxial substrate. The disorder caused by irradiation is mostly limited to increased widths of the existing U–O/U pair distributions, with any new neighbor shells being minor. As has been previously reported, the disorder caused by oxidative addition to U4O9 and U3O7 is much more extensive, resulting in multisite U–O distributions and greater reduction of the U–U amplitude with different distributions in bulk and thin-film U4O9. This includes the significant spectral feature near R = 1.2 Å for all U4O9 and U3O7 samples fit with a U-oxo type moiety with a U–O distance around 1.7 Å. In addition to indicating that these anomalies only occur in mixed valence materials, this work confirms the continuous rearrangement of the U–O distributions from 10 to 250 K. Although these variations of the structure are not observed in crystallography, their prominence in the EXAFS indicates that the dynamic structure underlying these effects is an essential factor of these materials.

Matteo Lo Verso, Carolina Introini, Luciana Barucca et al.

A complete understanding of the stability of fluid flows under varying magnetic field profiles is imperative for achieving control of plasma and operating fluids in the blankets of future fusion reactors. In this context, the primary objective of this study is to investigate the influence of varying magnetic profiles on the flow regime of a generic fluid, which is representative of both thermonuclear plasma and conductive fluids within a nuclear fusion reactor. To this aim in this work non-modal stability theory is adopted to perform stability analysis of a magneto-hydrodynamic (MHD) flow in an infinite circular pipe in order to study the effects of the magnetic field on the fluid dynamics of the pipe flow. In particular, the effects on the general stability of two magnetic field profiles are compared with the reference case of a pipe Poiseuille flow without magnetic field. Firstly, the classic modal stability technique is employed to study asymptotical stability. Then, non-modal stability analysis is applied to magneto-hydrodynamic pipe flow to study the system's response for a finite time immediately after a perturbation. Fourier–Chebyshev Petrov–Galerkin spectral method is used to compute the eigenvalues and pseudospectra of the weak formulation associated with the linearised system. Investigations on the dependence of spectra and transient growths on the specific magnetic profiles are conducted for different values of perturbation wave numbers. The obtained results show that in general the magnetic field has an effect of stabilization on the system, which depends on the specific magnetic profile considered. In addition, the non-modal stability analysis reveals that the inclusion of the magnetic field mitigates the effects of perturbations also in the short term, a phenomenon that cannot be seen using only modal stability analysis.

Samyak Jain, Peter J. Bruggeman

The penetration and propagation of streamers in capillary tubes is critical for applications involving the plasma-enabled disinfection of medical devices like catheters and plasma catalysis. In this study, a guided streamer is generated in a pulsed plasma jet operating in helium and impinged downstream onto a capillary tube with an inner diameter between 75 and 500 µm. The threshold voltage required to start the penetration of the guided streamer into the capillary was determined for both positive and negative polarities, and we observed a time delay between the streamer striking the top of the capillary and its penetration, which was found to be larger for the positive than the negative streamer. The observed differences can be explained by the need to sustain an electric field large enough to generate a sufficient seed electron density in the capillary to launch the streamer. The reported results suggest that the electric field at the capillary inlet is likely reduced by the formation of strong surface ionization waves for positive streamers. Nonetheless, in the case of positive streamers, the formation of surface streamers along the outside of the capillary wall can enhance streamer penetration into the capillary and the streamer propagation speed.

Tetsutarou Oishi, Shigeru Morita, Masahiro Kobayashi et al.

The ergodic layer in the Large Helical Device (LHD) consists of stochastic magnetic fields exhibiting a three-dimensional structure that is intrinsically formed by helical coils. Spectroscopic diagnostics was employed in the extreme ultraviolet (EUV) and vacuum ultraviolet (VUV) wavelength ranges to investigate emission lines of carbon impurities in both hydrogen (H) and deuterium (D) plasmas, aiming to elucidate the impact of distinct bulk ions on impurity generation and transport in the edge plasmas of the LHD. The emission intensity of carbon CIII, CIV, CV, and CVI lines is significantly higher in the D plasma compared to the H plasma, indicating a greater sputtering rate of carbon materials in the D plasma, resulting in a higher quantity of carbon impurities originating from the divertor plates. A Doppler profile measurement of the second order of CIV line emission (1548.20 × 2 Å) was attempted using a 3 m normal-incidence VUV spectrometer in the edge plasma at a horizontally elongated plasma position. The flow velocity reaches its maximum value close to the outermost region of the ergodic layer, and the observed flow direction aligns with the friction force in the parallel momentum balance. The flow velocity increases with the electron density in H plasmas, suggesting that the friction force becomes more dominant in the force balance at higher density regimes. This leads to an increase in the impurity flow, which can contribute to the impurity screening. In contrast, the flow velocity in the D plasma is smaller than that in the H plasma. The difference in flow values between D and H plasmas, when the friction force term dominates in the momentum balance, could be attributed to the mass dependence of the thermal velocity of the bulk ions.

Louis E. McNamara, John T. Kelly, Abigail M. Waldron et al.

Uranium hexafluoride (UF6) is a commonly utilized material feedstock in uranium enrichment processes due to its high vapor pressure and ease of sublimation. When exposed to air, UF6 undergoes spontaneous hydrolysis to form uranyl fluoride (UO2F2) particulates which are utilized for the detection of undeclared nuclear activities by nuclear safeguards organizations. The kinetics of the hydrolysis reaction and how they relate to particle morphology of the product are still debated in the literature. Here, we report the direct, in situ observation of UF6 reaction intermediates by cooling the reaction to cryogenic temperatures to significantly reduce the rate of hydrolysis. The reaction is then observable by Fourier transform infrared (FTIR) spectroscopy. The conversion of UF6 to UOF4 is observed as well as several other bands associated with possible long lived intermediate complexes. Chemometrics are used to further elucidate the reaction pathway from UF6 to UO2F2.

Alfred YiuFai Wong, Chun-Ching Shih

Concepts of dynamic oscillations of positive and negative ions to enhance fusion reactions are examined in this paper. Collective oscillations of positive and negative ions produce large oscillating electrostatic fields and could provide a significant reduction of the Coulomb potential barrier between the two interacting species (such as hydrogen anion H− and B+ in the hydrogen-boron fusion reaction). The negative hydrogen ions can be produced by populating low-temperature electrons around the neutral hydrogen atoms in a rotation chamber. The existence of H− ensures the stability of the plasma and the effectiveness of fusion interactions between H− and B+. In this paper, theoretical analyses of such oscillations systems will be presented and the conditions for fusion enhancement are discussed.

Dirk Wünderlich, Rudi Riedl, Markus Fröschle et al.

The large (size: 1 m × 2 m) radio frequency (RF) driven negative ion sources for the neutral beam heating (NBI) systems of the future fusion experiment ITER will be operated at a low filling pressure of 0.3 Pa, in hydrogen or in deuterium. The plasma will be generated by inductively coupling an RF power of up to 800 kW into the source volume. Under consideration for future neutral beam heating systems, like the one for the demonstration reactor DEMO, is an even lower filling pressure of 0.2 Pa. Together with the effect of neutral gas depletion, such low operational pressures can result in a neutral gas density below the limit required for sustaining the plasma. Systematic investigations on the low-pressure operational limit of the half-ITER-size negative ion source of the ELISE (Extraction from a Large Ion Source Experiment) test facility were performed, demonstrating that operation is possible below 0.2 Pa. A strong correlation of the lower pressure limit on the magnetic filter field topology is found. Depending on the field topology, operation close to the low-pressure limit is accompanied by strong plasma oscillations in the kHz range.

Dariusz Korzec, Florian Hoppenthaler, Stefan Nettesheim

The piezoelectric direct discharge (PDD) is a comparatively new type of atmospheric pressure gaseous discharge for production of cold plasma. The generation of such discharge is possible using the piezoelectric cold plasma generator (PCPG) which comprises the resonant piezoelectric transformer (RPT) with voltage transformation ratio of more than 1000, allowing for reaching the output voltage >10 kV at low input voltage, typically below 25 V. As ionization gas for the PDD, either air or various gas mixtures are used. Despite some similarities with corona discharge and dielectric barrier discharge, the ignition of micro-discharges directly at the ceramic surface makes PDD unique in its physics and application potential. The PDD is used directly, in open discharge structures, mainly for treatment of electrically nonconducting surfaces. It is also applied as a plasma bridge to bias different excitation electrodes, applicable for a broad range of substrate materials. In this review, the most important architectures of the PDD based discharges are presented. The operation principle, the main operational characteristics and the example applications, exploiting the specific properties of the discharge configurations, are discussed. Due to the moderate power achievable by PCPG, of typically less than 10 W, the focus of this review is on applications involving thermally sensitive materials, including food, organic tissues, and liquids.