The enhancement of photocatalytic hydrogen production via Ti3+ self-doping black TiO2/g-C3N4 hollow core-shell nano-heterojunction
Abstrak
Abstract The Ti3+ self-doping B-TiO2/g-C3N4 hollow core-shell nano-heterojunction is synthesized via the continuous hydrothermal deposition and sculpture-reduction processes. The results of SEM, XRD, TEM, XPS and FT-IR imply that the B-TiO2/g-C3N4 hollow core-shell nanospheres have been prepared successfully. The photocatalytic activity of the B-TiO2/g-C3N4 nano-heterojunctions remarkably exhibits an enhancement of 18 times and 65 times than that of normal TiO2 and g-C3N4, respectively. Further, the photocatalytic process and the mechanism of the photocatalytic hydrogen production enhancement have been studied, which could be ascribed to the Ov-Ti3+ in the B-TiO2 and interface nano-heterojunction, that have been proved by the transient photocurrent, PL, EIS and Mott-Schottky plots.
Topik & Kata Kunci
Penulis (9)
Jiaqi Pan
Zongjun Dong
Beibei Wang
Ziyuan Jiang
Chuang Zhao
Jingjing Wang
Changsheng Song
Yingying Zheng
Chaorong Li
Akses Cepat
PDF tidak tersedia langsung
Cek di sumber asli →- Tahun Terbit
- 2019
- Bahasa
- en
- Total Sitasi
- 463×
- Sumber Database
- Semantic Scholar
- DOI
- 10.1016/J.APCATB.2018.09.079
- Akses
- Open Access ✓