Semantic Scholar Open Access 2024 28 sitasi

Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser

Zhaoheng Guo T. Driver S. Beauvarlet D. Cesar J. Duris +107 lainnya

Lihat Sumber

Abstrak

Pump-probe experiments with sub-femtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of sub-femtosecond pulse pairs from a two-colour X-ray free-electron laser (XFEL). By measuring the delay between the two pulses with an angular streaking diagnostic, we characterise the group velocity of the XFEL and demonstrate control of the pulse delay down to 270 as. We demonstrate the application of this technique to a pump-probe measurement in core-excited para-aminophenol. These results demonstrate the ability to perform pump-probe experiments with sub-femtosecond resolution and atomic site specificity.

Topik & Kata Kunci

Physics

Penulis (112)

Zhaoheng Guo

T. Driver

S. Beauvarlet

D. Cesar

J. Duris

P. Franz

O. Alexander

D. Bohler

C. Bostedt

V. Averbukh

Xinxin Cheng

L. DiMauro

G. Doumy

R. Forbes

O. Gessner

J. Glownia

Erik Isele

A. Kamalov

K. Larsen

Siqi Li

Xiang Li

Ming-Fu Lin

G. McCracken

R. Obaid

Jordan T. ONeal

R. Robles

D. Rolles

M. Ruberti

A. Rudenko

D. S. Slaughter

N. Sudar

E. Thierstein

D. Tuthill

K. Ueda

Enliang Wang

Anna L. Wang

Jun Wang

T. Weber

T. Wolf

Linda Young

Zhen Zhang

P. Bucksbaum

J. Marangos

Matthias F. Kling

Zhirong Huang

Peter Walter

L. Inhester

N. Berrah

J. Cryan

A. S. A. N. Laboratory

Menlo Park

CA 94025

Usa

D. Physics

Stanford University

Stanford

USA. Department of physics

Stanford Pulse Institute

S. N. Laboratory

Linac Coherent Light Source

Usa Department of Computer Science

Physics Department

U. O. Connecticut

Storrs

CT 06269

Center for Free-Electron Laser Science Cfel

D. E. Desy

85 Notkestr.

21029 Hamburg

Germany.

Quantum Optics

Laser Science Group

B. Laboratory

I. -. London

London

SW7 2BW

United Kingdom.

D. Physics

The Pennsylvania State University

Columbus

OH 43210

D. Chemistry

Tohoku University

Sendai 980-8578

Japan.

James Franck Institute

The University of Chicago

Chicago

C. Division

Lawrence Berkeley National Laboratory

Berkeley

CA 94720

Usa J.R. Macdonald Laboratory

Kansas State University

Manhattan

Kansas 66506

Usa Chemical Sciences

Engineering Division

A. N. Laboratory

Argonne

60439

Usa Paul-Scherrer Institute

CH-5232

Villigen Psi

Switzerland Institute for Nuclear Research of the Russian Acad Sciences

Institute of Space Sciences

Engineering

E. P. F. Lausanne

CH-1015

Lausanne

Switzerland.

Format Sitasi

APA MLA BibTeX

Guo, Z., Driver, T., Beauvarlet, S., Cesar, D., Duris, J., Franz, P. et al. (2024). Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser. https://www.semanticscholar.org/paper/37c6214deb3f8b3e97d7f393e1ccd50326a63954

@article{guo2024, author = {Zhaoheng Guo and T. Driver and S. Beauvarlet and D. Cesar and J. Duris and P. Franz and O. Alexander and D. Bohler and C. Bostedt and V. Averbukh and Xinxin Cheng and L. DiMauro and G. Doumy and R. Forbes and O. Gessner and J. Glownia and Erik Isele and A. Kamalov and K. Larsen and Siqi Li and Xiang Li and Ming-Fu Lin and G. McCracken and R. Obaid and Jordan T. ONeal and R. Robles and D. Rolles and M. Ruberti and A. Rudenko and D. S. Slaughter and N. Sudar and E. Thierstein and D. Tuthill and K. Ueda and Enliang Wang and Anna L. Wang and Jun Wang and T. Weber and T. Wolf and Linda Young and Zhen Zhang and P. Bucksbaum and J. Marangos and Matthias F. Kling and Zhirong Huang and Peter Walter and L. Inhester and N. Berrah and J. Cryan and A. S. A. N. Laboratory and Menlo Park and CA 94025 and Usa and D. Physics and Stanford University and Stanford and USA. Department of physics and Stanford Pulse Institute and S. N. Laboratory and Linac Coherent Light Source and Usa Department of Computer Science and Physics Department and U. O. Connecticut and Storrs and CT 06269 and Center for Free-Electron Laser Science Cfel and D. E. Desy and 85 Notkestr. and 21029 Hamburg and Germany. and Quantum Optics and Laser Science Group and B. Laboratory and I. -. London and London and SW7 2BW and United Kingdom. and D. Physics and The Pennsylvania State University and Columbus and OH 43210 and D. Chemistry and Tohoku University and Sendai 980-8578 and Japan. and James Franck Institute and The University of Chicago and Chicago and Il and C. Division and Lawrence Berkeley National Laboratory and Berkeley and CA 94720 and Usa J.R. Macdonald Laboratory and Kansas State University and Manhattan and Kansas 66506 and Usa Chemical Sciences and Engineering Division and A. N. Laboratory and Argonne and 60439 and Usa Paul-Scherrer Institute and CH-5232 and Villigen Psi and Switzerland Institute for Nuclear Research of the Russian Acad Sciences and Institute of Space Sciences and Engineering and E. P. F. Lausanne and CH-1015 and Lausanne and Switzerland.}, title = {Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser}, year = {2024}, journal = {Semantic Scholar}, url = {https://www.semanticscholar.org/paper/37c6214deb3f8b3e97d7f393e1ccd50326a63954}, }

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Informasi Jurnal

Tahun Terbit: 2024
Bahasa: en
Total Sitasi: 28×
Sumber Database: Semantic Scholar
Akses: Open Access ✓