Preparation and Transport Properties of Mn_2.16Ga Single Crystal

In recent years, antiferromagnetic kagome materials have attracted considerable attention in condensed matter physics owing to their distinctive lattice geometry. In this work, high-quality single crystals of D019-structured Mn_2.16Ga were grown using the flux method, and their magnetotransport properties were systematically studied. Measurements of magnetization versus field (M–H), temperature-dependent magnetization (M–T), and the anomalous Hall effect confirm that the crystal undergoes a magnetic-structural transition driven by both temperature and the magnetic field. Remarkably, a coexistence of positive and negative longitudinal magnetoresistance (MR) is observed in Mn_2.16Ga. The MR shows a field-induced sign change from negative to positive. The negative MR is attributed to field-modified magnetic ordering, whereas the positive MR originates mainly from interlayer electron conduction in the kagome lattice and distortion of the in-plane triangular arrangement of Mn magnetic moments. These results offer valuable insights into the electronic and magnetic transport behavior of Mn-based antiferromagnetic single crystals.