DOAJ Open Access 2024

Self-healing and shape-memory polymers based on cellulose acetate matrix

Han Jia Keiya Jimbo Hirogi Yokochi Hideyuki Otsuka Tsuyoshi Michinobu

Abstrak

The creation of self-healing polymers with superior strength and stretchability from biodegradable materials is attracting increasing attention. In this study, we synthesized new biomass-derived cellulose acetate (CA) derivatives by ring-opening graft polymerization of δ-valerolactone followed by the introduction of ureidopyrimidinone (Upy) groups in the polymer side chains. Due to the semicrystalline aliphatic characteristics of the side chain poly(δ-valerolactone) (PVL) and quadruple hydrogen bonds formed by the Upy groups, the stretchability of the resulting polymers was significantly enhanced. Moreover, the shape memory ability and self-healing property (58.3% of self-healing efficiency) were successfully imparted to the polymer. This study demonstrates the great significance of using biomass sources to create self-healing polymers.

Penulis (5)

H

Han Jia

K

Keiya Jimbo

H

Hirogi Yokochi

H

Hideyuki Otsuka

T

Tsuyoshi Michinobu

Format Sitasi

Jia, H., Jimbo, K., Yokochi, H., Otsuka, H., Michinobu, T. (2024). Self-healing and shape-memory polymers based on cellulose acetate matrix. https://doi.org/10.1080/14686996.2024.2320082

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Informasi Jurnal
Tahun Terbit
2024
Sumber Database
DOAJ
DOI
10.1080/14686996.2024.2320082
Akses
Open Access ✓