DOAJ Open Access 2022

Bi-MOFs with two different morphologies promoting degradation of organic dye under simultaneous photo-irradiation and ultrasound vibration treatment

Shanghai Dong Liying Wang Weiyi Lou Yunxin Shi Zhenzhu Cao +2 lainnya

Abstrak

For the first time, piezocatalysis activity has been observed in bismuth-based MOFs (ultrasound vibration treatment) with two different morphologies, namely FCAU-17 (flakes) and CAU-17 (rods). CAU-17 and FCAU-17 were synthesized by solvothermal and ultrasonic methods, respectively, with the same organic ligand (1,3,5-benzenetricarboxylic acid) and metal salt (Bi(NO3)3·5H2O). Among these, the apparent rate constant k of CAU-17 in piezo-photocatalysis is 3.9 × 10−2 min−1, which is ∼3.9 and ∼ 1.5 times of those in photocatalysis and piezocatalysis, respectively. CAU-17 showed much high piezo-photocatalytic activity during degradation of RhB. Efficiently coupling between piezocatalysis and photocatalysis has been realized in rod-like CAU-17 (ultrasound vibration treatment). Our results provide a new strategy to improve catalytic performance of Bi MOFs through an efficient synergistic piezo-photocatalysis approach for environmental remediation.

Penulis (7)

S

Shanghai Dong

L

Liying Wang

W

Weiyi Lou

Y

Yunxin Shi

Z

Zhenzhu Cao

Y

Yongfeng Zhang

J

Junmin Sun

Format Sitasi

Dong, S., Wang, L., Lou, W., Shi, Y., Cao, Z., Zhang, Y. et al. (2022). Bi-MOFs with two different morphologies promoting degradation of organic dye under simultaneous photo-irradiation and ultrasound vibration treatment. https://doi.org/10.1016/j.ultsonch.2022.106223

Akses Cepat

Informasi Jurnal
Tahun Terbit
2022
Sumber Database
DOAJ
DOI
10.1016/j.ultsonch.2022.106223
Akses
Open Access ✓