A pathway towards decentralized studies of radioactive post-lead elements and their applications in beyond standard model physics
Abstrak
Molecules have proven to be sensitive tools for studying physics beyond the standard model, with heavy and deformed nuclei offering decisive sensitivity to parity- and time-reversal-violating effects. However, almost all elements beyond lead, occupying the 6p~to~5f atomic orbitals, lack stable isotopes, hence molecules containing them are referred to as radioactive molecules. Among those, radium monofluoride has seen particular interest, but to date, research on radioactive molecules has mainly been limited to large-scale nuclear facilities. Here, we present a scheme that allows efficient and fast harvest of radioactive ions (including short-lived Ra), and show ion gas-phase reaction studies of singly and doubly charged Ra, Po, and Pb ions with SF$_6$ gas inside an ion trap. Our results show that the chemical reaction rate of Ra$^+$ is in line with trends of other alkaline earth elements, further support by quantum chemical computations. The reaction Ra$^{2+}$ + SF$_6$ $\rightarrow$ RaF${^+}$ + SF$_5^{+}$ achieves an almost unity conversion efficiency, making it particularly suitable for the application for studies in physics beyond the standard model. The scheme enables future decentralized research avenues with short-lived radioactive molecules for fundamental physics research at laboratories without the need for local nuclear reactors or accelerators.
Topik & Kata Kunci
Penulis (24)
Moritz Pascal Reiter
Kriti Mahajan
Meetika Narang
Carsten Zuelch
Timo Dickel
Daler Amanbayev
Robert Berger
Julian Bergmann
Agnieszka Bukowicka
Mariam Fadel
Tayemar Fowler-Davies
Zhuang Ge
Simeon Gloeckner
Gabriella Kripko-Koncz
Nasser Kalantar-Nayestanaki
Cameron Merron
David J. Morrissey
Wolfgang Plass
Christoph Scheidenberger
Makar Simonov
Nazarena Tortorelli
Jiajun Yu
Alexandra Zadvornaya
Jianwai Zhao
Akses Cepat
- Tahun Terbit
- 2025
- Bahasa
- en
- Sumber Database
- arXiv
- Akses
- Open Access ✓