arXiv Open Access 2025

Superconductivity emerging from the N${é}$el state in ${\it infinite}$-${\it stage}$ single-layer cuprate La$_2$CuO$_{4+δ}$

Yoshihiko Ihara Ramender Kumar Kota Miyakoshi Migaku Oda Kenji Ishida
Lihat Sumber

Abstrak

In copper oxides (cuprates) with single CuO$_2$ layer such as La$_{2-x}$Ba(Sr)$_x$CuO$_4$, antiferromagnetism coexists with superconductivity at small doping levels $x$, where chemical disorders are significant. Here, we report that superconductivity occurs in a uniform and fully ordered N${é}$el state in a single-layer cuprate La$_2$CuO$_{4+δ}$ with a small amount of excess oxygen $(δ= 0.015)$ as demonstrated by the $^{139}$La nuclear quadrupole resonance measurement. A uniform oxygen distribution in the crystal is crucial for achieving microscopic phase coexistence and overcoming the miscibility gap associated with the staging instability; self-organized periodic oxygen arrangement driven by mobile oxygen atoms. This finding prompts the reconsideration of superconductivity in cuprates, highlighting that it can emerge in a robust N${é}$el state that retains sizable magnetic moments and hosts only a small carrier density.

Penulis (5)

Y

Yoshihiko Ihara

R

Ramender Kumar

K

Kota Miyakoshi

M

Migaku Oda

K

Kenji Ishida

Format Sitasi

Ihara, Y., Kumar, R., Miyakoshi, K., Oda, M., Ishida, K. (2025). Superconductivity emerging from the N${é}$el state in ${\it infinite}$-${\it stage}$ single-layer cuprate La$_2$CuO$_{4+δ}$. https://arxiv.org/abs/2507.20138

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2025
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en
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arXiv
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Open Access ✓